Мое отработанное решение. Проверено на 1000+ раз:
public static long RandomLong(long min, long max)
{
return min + (long)RandomULong(0, (ulong)Math.Abs(max - min));
}
public static ulong RandomULong(ulong min, ulong max)
{
var hight = Rand.Next((int)(min >> 32), (int)(max >> 32));
var minLow = Math.Min((int)min, (int)max);
var maxLow = Math.Max((int)min, (int)max);
var low = (uint)Rand.Next(minLow, maxLow);
ulong result = (ulong)hight;
result <<= 32;
result |= (ulong)low;
return result;
}