Сначала сожмите свои массивы:
In [1]: import numpy as np
In [2]: keys = np.array(
...: [[' THE OLD TESTAMENT '],
...: [' SEAN SONG '],
...: [' CITY WALK ']]
...: )
In [3]: values = np.array(
...: [[' This is the name of an Old Testament '],
...: [' Hello this is great '],
...: [' Wait the way you are doing ']]
...: )
In [4]: dict(zip(keys.squeeze(), values.squeeze()))
Out[4]:
{' CITY WALK ': ' Wait the way you are doing ',
' SEAN SONG ': ' Hello this is great ',
' THE OLD TESTAMENT ': ' This is the name of an Old Testament '}
Или просто используйте нарезку:
In [5]: dict(zip(keys[:,0], values[:,0]))
Out[5]:
{' CITY WALK ': ' Wait the way you are doing ',
' SEAN SONG ': ' Hello this is great ',
' THE OLD TESTAMENT ': ' This is the name of an Old Testament '}