Для описываемого вами случая не требуется никакой петли:
set.seed(42)
mat <- matrix(sample(0:1, 100, replace = T), ncol=10)
mat.ind <- which(mat==T, arr.ind=T)
> mat
[,1] [,2] [,3] [,4] [,5] [,6] [,7] [,8] [,9] [,10]
[1,] 1 0 1 1 0 0 1 0 1 1
[2,] 1 1 0 1 0 0 1 0 0 0
[3,] 0 1 1 0 0 0 1 0 0 0
[4,] 1 0 1 1 1 1 1 0 1 1
[5,] 1 0 0 0 0 0 1 0 1 1
[6,] 1 1 1 1 1 1 0 1 1 1
[7,] 1 1 0 0 1 1 0 0 0 0
[8,] 0 0 1 0 1 0 1 0 0 1
[9,] 1 0 0 1 1 0 1 1 0 1
[10,] 1 1 1 1 1 1 0 0 0 1
> mat.ind
row col
[1,] 1 1
[2,] 2 1
[3,] 4 1
[4,] 5 1
[5,] 6 1
[6,] 7 1
... ... ...